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Ethanol and benzene extractive distillation simulation on DWSIM utilizing p-xylene as solvent

K. Laturkar, Facility for Rare Isotope Beams, Michigan State University, East Lansing, Michigan (U.S.); and K. LATURKAR, Validation Associates LLC, Framingham, Massachusetts (U.S.)

A boiling liquid mixture is subjected to distillation to separate its components according to their different volatilities.1 In situations where the boiling points of components of a mixture are close to each other, extractive distillation can be used rather than simple distillation. In extractive distillation, a non-volatile solvent is used—this alters the relative volatility of the components without forming an azeotropic mixture with them.2 The extractive distillation process utilizes the selective accentuation of the non-ideal characteristics of the liquid phase components to be separated that are induced by the presence of solvent. The solvent achieves this by altering the activity coefficient of the individual components.3

These newly formed solvent-component mixtures can then be separated using normal distillation. The individual mixtures once separated out as products from the process can then be purified in another distillation column to separate the solvent from the components. This solvent can then be recycled back into the first column along with fresh solvent. To quantify the risks associated with different parameter settings in a model and optimize the system, a sensitivity analysis can be performed. This is a valuable tool for understanding the model's strengths and weaknesses and can be utilized to recommend operational approaches for the system.

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Theory. Extractive distillation must adhere to certain guidelines to be effective:3

  1. Solvent presence in the liquid phase should influence the key components differently for improved separation.
  2. To remain predominantly in liquid phase, the non-volatile solvent must boil at a higher temperature than the key components of the separation.
  3. Azeotropes should not be produced between the solvent and the components in the mixture to be separated.
  4. The solvent feed should be placed above the primary feed in dual-feed extractive columns. The extractive section will distill out the light key component while the bottoms will consist of a mixture of the heavy key component and the solvent.

For this article, the separation of an ethanol and benzene mixture is considered. Ethanol and benzene—with their boiling points of 78.24°C and 80.08°C, respectively4—are difficult to separate using normal distillation. To separate them, p-xylene with its relatively high boiling point of 138.3°C is used as a solvent in a dual-feed distillation column.4 It reacts with ethanol and benzene in a way so that the benzene and p-xylene mixture separates out from the bottom while relatively pure ethanol is taken out from the top. This benzene and p-xylene mixture is then sent to a solvent recovery distillation column where both components are separated out and the p-xylene is recycled back into the first distillation column as solvent. A simulation study was conducted using the process simulator DWSIM, an open source software to simulate steady-state operations.5 Input conditions for the above mentioned operation were entered into the software to analyze the process.

FIG. 1 shows the T-xy plot for the minimum boiling ethanol-benzene azeotropic mixture with an azeotropic temperature of around 314 K, which makes it difficult to separate using simple distillation methods.6 As shown in the diagram, a relatively flat region is found near the minimum on the bubble point curve, which slopes gently in both directions. With increasing distance from the intersection point, these slopes become steeper. As for the dewpoint curve, a relatively constant slope characterizes it between the azeotropic and pure component points.7

Laturkar-Fig-01

Mathematical model. An equilibrium stage model (EQ) is considered for the extractive distillation process. One EQ stage corresponds to one section of tray or packaging, depending on the type of column. To develop this model, certain assumptions must be made, as outlined here:8

  1. A steady-state condition is reached.
  2. Mechanical equilibrium is attained by the system.
  3. Vapor and liquid phases are positioned at phase equilibrium and assumed to be perfectly mixed.
  4. Heat generated during mixing is neglected.
  5. Only liquid-phase reactions are considered.
  6. Both the reboiler and condenser represent stages at equilibrium.
  7. All stages are at equilibrium if chemical reactions are considered.
  8. Equilibrium caused by chemical reactions is not accounted for in every stage if no chemical reactions are considered.

FIG. 2 represents the EQ stage model schematically. The mathematical model for the extractive distillation process at a particular stage in the column is given by the equations below.9

Laturkar-Fig-02

The mass balance across an EQ stage is given by Eq. 1:

Laturkar Equ 01

When hold-up of vapor is not considered in the EQ stage, the material balance for the components is determined by Eq. 2:

Laturkar Equ 02

The sidestream-to-interstage flow ratio for the vapor and liquid phases is (Eq. 3):

Laturkar Equ 03

To relate the equilibrium between the vapor and liquid phases, Eq. 4 is used:

Laturkar Equ 04

where (Eq. 5):

Laturkar Equ 05

The equation of enthalpy balance across an EQ stage is shown in Eq. 6:

Laturkar Equ 06

All time derivatives in the above equations are zero since the process is said to occur under steady-state conditions. Additionally, since the various components do not react, the reaction rates also remain zero.

CASE STUDY MODELING ON DWSIM

An equimolar azeotropic mixture of benzene and ethanol at the rate of 100 kmol/hr (1 atm and 298.15 K) is fed into a 71-tray extractive distillation column on Tray 50.10 The makeup solvent, which consists of pure p-xylene, is fed at a flowrate of 0.301 kmol/hr (1 atm and 298.15 K) to a static mixer and is mixed with the recycle stream from the solvent recovery column. The outlet of this mixture is fed to the extractive distillation column on Tray 24. With a reflux ratio of 2.13, the lighter product distills out from the top and contains ethanol as the key component, while the bottoms is a mixture of benzene and p-xylene with the benzene mol fraction at 0.189. The bottoms product is then sent to a 21-tray solvent recovery column where it enters the column on Tray 8. In this simple distillation where the reflux ratio is 6.14, benzene is separated as the top product and p-xylene distills out from the bottom. The bottoms stream from the solvent recovery column is passed through a cooler, where it is cooled to a temperature of 100°C before being recycled and fed into the static mixer.

FIG. 3 shows the flowsheet of the entire process. The products shown in parentheses are the main key components of that stream.

Laturkar-Fig-03

The simulation was conducted using the UNIversal QUAsi‐Chemical (UNIQUAC) activity coefficients in a DWSIM process simulator.11 For simplicity, the whole system was considered to be at a constant pressure of 1 atm without any pressure drop. For both of the extractive distillation and solvent recovery columns, the K-value model used was DECHEMA, with the ideal gas as the equation of state and Antoine equation used for the vapor pressure relations.12 In the absence of solvent recycle flowrate information in the problem, an initial estimate of 200 kmol/hr was made before beginning the simulation.

Results and discussions. The simulation was performed after initializing the parameters to carry out the steady-state operation. TABLE 1 shows the specifications for this process and the simulation results. The stages are numbered in descending order, with the first stage at the top. The reboiler and condenser are considered as stages in both the columns.

Laturkar Table 01

FIG. 4 illustrates the composition profile across the extractive distillation column. An analysis of the curve indicates that the composition of ethanol is highest at the top of the column: the lighter key component with a mole fraction of 0.7355. Trace quantities (mole fraction 0.0045) of p-xylene are also present in the distillate. Another fractionating column can be used to further refine this distillate. The bottom fraction contains very small amounts of ethanol. The majority is a mixture of p-xylene (mol fraction 0.811) and benzene (mol fraction 0.189) which is then sent to the solvent recovery column as feed.

Laturkar-Fig-04

The composition profile of the solvent recovery column is shown in FIG. 5. Based on the fact that the column feed only had trace amounts of ethanol, both the distillate and bottoms contain minimal amounts of ethanol. Benzene (mol fraction 0.99) is distilled from the top of the column while p-xylene (mol fraction 0.933) is taken from the bottom. The bottoms from this column are then recycled back at the rate of 214.697 kmol/hr (calculated in the simulation), where it combines with fresh solvent before being fed to the first column.

Laturkar-Fig-05

Sensitivity analysis study. An analysis of the system's sensitivity is performed by varying parameters of the process, such as flowrate and mole fraction, to understand how the changes affect ethanol outlet parameters over specified intervals.

Case 1: Variation of ethanol production with the mass flowrate of the makeup stream. FIG. 6 shows the flowrate of ethanol production as a function of the makeup stream flowrate. This flowrate varies between 15 kg/hr and 50 kg/hr without affecting any other parameters. From the figure, it is evident that the highest production of ethanol occurs around 30 kg/hr of the makeup stream. Increasing the makeup stream can increase the quantity of ethanol produced only up to a certain point. The column will be more mass- and heat-laden after that point, but no extra separation will occur.

Laturkar-Fig-06

Case 2: Variation of the ethanol production rate and mole fraction with the change in solvent mole fraction. A change in the concentration of p-xylene in the solvent used for the first column can be utilized to examine the changes in two parameters, namely mole fraction and production rate of ethanol. FIG. 7 shows the effects of varying the solvent mole fraction of p-xylene from 0.85 to 0.99. As the p-xylene concentration increases, the ethanol production rate decreases, while the mole fraction of ethanol in the distillate increases. Ideal operation of the column can be achieved by considering the intersection as an optimum point between production and purity. The final operation will be determined by the process requirements, and such tools will aid in optimizing the process.

Laturkar-Fig-07

Takeaway. Azeotrope mixtures of ethanol and benzene can be separated with p-xylene utilizing the extractive distillation method. By using the UNIQUAC thermodynamic model, a steady-state simulation was performed on DWSIM software using p-xylene as a solvent to separate the ethanol-benzene mixture. The simulation demonstrated that ultrapure benzene can be produced in two consecutive distillation columns and a majority of the solvent (p-xylene) can be recovered and recycled back into the process. Using sensitivity analysis, certain parameters can be modified to increase the flowrate of components or enhance purity. System response can be observed by changing other parameters such as reflux ratios, feed tray placement, feed temperatures, feed pressures, reboiler duty, etc. Additionally, it may also be possible to investigate the use of other solvents for better separation of the components. HP

ACKNOWLEDGEMENT

The authors are grateful to Muhammad Saif for being the inspiration for this work.10

NOMENCLATURE

Laturkar Nomenclature

LITERATURE CITED

  1. Kister, H. Z., Distillation Design, McGraw-Hill Inc., 1992.
  2. Gerbaud, V., I. Rodriguez-Donis, L. Hegely, P. Lang, F. Denes and X. You, "Review of extractive distillation. Process design, operation, optimization and control," Chemical Engineering Research and Design, Vol. 141, January 2019.
  3. Perry, R. H. and D. W. Green, "Distillation,” Perry’s Chemical Engineers' Handbook, 9th Ed., The McGraw-Hill Co. Inc., 1999.
  4. Haynes, W. M., CRC Handbook of Chemistry and Physics, 97th Ed., CRC Press, Taylor & Francis Group, 2016–2017.
  5. DWSIM, "Chemical process simulation for everyone," DWSIM, online: https://dwsim.org/
  6. Goral, M., A. Skrzecz, A. Bok, A. Maczynski and P. Oracz, "Recommended vapor–liquid equilibrium data. Part 3: Binary alkanol–aromatic hydrocarbon systems," Journal of Physical and Chemical Reference Data, Vol. 33, No. 3, September 2004.
  7. Hadler, A. B., L. S. Ott and T. J. Bruno, "Study of azeotropic mixtures with the advanced distillation curve approach," Fluid Phase Equilibria, Vol. 281, No. 1, 2009.
  8. Lei, Z., C. Li, Y. Li and B. Chen, "Separation of acetic acid and water by complex extractive distillation," Separation and Purification Technology, Vol. 36, No. 2, 2004.
  9. Lei, Z., C. Li and B. Chen, "Extractive distillation: A review," Separation & Purification Reviews, Vol. 32, No. 2, 2003.
  10. Saif, M., “Extractive distillation of ethanol and benzene using p-xylene in DWSIM,” 2021, online: https://www.youtube.com/watch?v=1oHuEmsIRvA
  11. Abrams, D. S. and J. M. Prausnitz, "Statistical thermodynamics of liquid mixtures: A new expression for the excess Gibbs energy of partly or completely miscible systems," AIChE Journal, Vol. 21, No. 1, 1975.
  12. "Fugacity," cocosimulator.org, 2021, online: https://www.cocosimulator.org/index_help.php?page=TEA/fugacity.htm
First Author Rule Line
Author-pic-Kaustubh

KAUSTUBH LATURKAR works as an Engineer at the Facility for Rare Isotope Beams, a U.S. Department of Energy (DOE) project in Michigan. He has more than 9 yr of experience working in the field of process engineering, refinery operations, utility systems design and operation, with a special focus on design and commissioning of engineering systems. Laturkar earned an MS degree in chemical engineering from University of Florida and a BE degree in chemical engineering from Panjab University, Chandigarh, India. The author can be reached at kos19188@gmail.com.

Author-pic-Kasturi

KASTURI LATURKAR works as a Validation Engineer for Validation Associates LLC and has more than 4 yr of experience working in commissioning, qualification and validation of upstream and downstream bioprocessing equipment and critical utilities. Laturkar graduated with an MS degree in chemical engineering from Syracuse University and a B.Tech degree in chemical engineering from Guru Gobind Singh Indraprastha University, Delhi, India. The author can be reached at kasturi.laturkar@gmail.com.